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Review-SEI: Past, Present and Future

Journal of the Electrochemical Society, 2017-01, Vol.164 (7), p.A1703-A1719 [Peer Reviewed Journal]

The Author(s) 2017. Published by ECS. ;EISSN: 1945-7111 ;DOI: 10.1149/2.1441707jes

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  • Title:
    Review-SEI: Past, Present and Future
  • Author: Peled, E. ; Menkin, S.
  • Is Part Of: Journal of the Electrochemical Society, 2017-01, Vol.164 (7), p.A1703-A1719
  • Description: The Solid-Electrolyte-Interphase (SEI) model for non-aqueous alkali-metal batteries constitutes a paradigm change in the understanding of lithium batteries and has thus enabled the development of safer, durable, higher-power and lower-cost lithium batteries for portable and EV applications. Prior to the publication of the SEI model (1979), researchers used the Butler-Volmer equation, in which a direct electron transfer from the electrode to lithium cations in the solution is assumed. The SEI model proved that this is a mistaken concept and that, in practice, the transfer of electrons from the electrode to the solution in a lithium battery, must be prevented, since it will result in fast self-discharge of the active materials and poor battery performance. This model provides [E. Peled, in "Lithium Batteries," J.P. Gabano (ed), Academic Press, (1983), E. Peled, J. Electrochem. Soc., 126, 2047 (1979).] new equations for: electrode kinetics (io and b), anode corrosion, SEI resistivity and growth rate and irreversible capacity loss of lithium-ion batteries. This model became a cornerstone in the science and technology of lithium batteries. This paper reviews the past, present and the future of SEI batteries.
  • Publisher: The Electrochemical Society
  • Language: English
  • Identifier: EISSN: 1945-7111
    DOI: 10.1149/2.1441707jes
  • Source: IOPscience (Open Access)
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