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Ruthenium-Catalyzed CC Bond Cleavage in Lignin Model Substrates

Angewandte Chemie (International ed.), 2015-05, Vol.54 (20), p.5859 [Peer Reviewed Journal]

2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim ;ISSN: 1433-7851 ;EISSN: 1521-3773 ;DOI: 10.1002/anie.201410620 ;CODEN: ACIEAY

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  • Title:
    Ruthenium-Catalyzed CC Bond Cleavage in Lignin Model Substrates
  • Author: vomStein, Thorsten ; denHartog, Tim ; Buendia, Julien ; Stoychev, Spas ; Mottweiler, Jakob ; Bolm, Carsten ; Klankermayer, Jurgen ; Leitner, Walter
  • Subjects: Lignin
  • Is Part Of: Angewandte Chemie (International ed.), 2015-05, Vol.54 (20), p.5859
  • Description: Ruthenium-triphos complexes exhibited unprecedented catalytic activity and selectivity in the redox-neutral CC bond cleavage of the [beta]-O-4 lignin linkage of 1,3-dilignol model compounds. A mechanistic pathway involving a dehydrogenation-initiated retro-aldol reaction for the CC bond cleavage was proposed in line with experimental data and DFT calculations.
  • Publisher: Weinheim: Wiley Subscription Services, Inc
  • Language: English
  • Identifier: ISSN: 1433-7851
    EISSN: 1521-3773
    DOI: 10.1002/anie.201410620
    CODEN: ACIEAY
  • Source: Alma/SFX Local Collection
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