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Chiral light intrinsically couples to extrinsic/pseudo-chiral metasurfaces made of tilted gold nanowires

Scientific reports, 2016-08, Vol.6 (1), p.31796-31796, Article 31796 [Peer Reviewed Journal]

Copyright Nature Publishing Group Aug 2016 ;Copyright © 2016, The Author(s) 2016 The Author(s) ;ISSN: 2045-2322 ;EISSN: 2045-2322 ;DOI: 10.1038/srep31796 ;PMID: 27553888

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  • Title:
    Chiral light intrinsically couples to extrinsic/pseudo-chiral metasurfaces made of tilted gold nanowires
  • Author: Belardini, Alessandro ; Centini, Marco ; Leahu, Grigore ; Hooper, David C ; Li Voti, Roberto ; Fazio, Eugenio ; Haus, Joseph W ; Sarangan, Andrew ; Valev, Ventsislav K ; Sibilia, Concita
  • Subjects: Circular dichroism ; Gold ; Nanotechnology ; Nanowires ; Polarized light
  • Is Part Of: Scientific reports, 2016-08, Vol.6 (1), p.31796-31796, Article 31796
  • Description: Extrinsic or pseudo-chiral (meta)surfaces have an achiral structure, yet they can give rise to circular dichroism when the experiment itself becomes chiral. Although these surfaces are known to yield differences in reflected and transmitted circularly polarized light, the exact mechanism of the interaction has never been directly demonstrated. Here we present a comprehensive linear and nonlinear optical investigation of a metasurface composed of tilted gold nanowires. In the linear regime, we directly demonstrate the selective absorption of circularly polarised light depending on the orientation of the metasurface. In the nonlinear regime, we demonstrate for the first time how second harmonic generation circular dichroism in such extrinsic/pseudo-chiral materials can be understood in terms of effective nonlinear susceptibility tensor elements that switch sign depending on the orientation of the metasurface. By providing fundamental understanding of the chiroptical interactions in achiral metasurfaces, our work opens up new perspectives for the optimisation of their properties.
  • Publisher: England: Nature Publishing Group
  • Language: English
  • Identifier: ISSN: 2045-2322
    EISSN: 2045-2322
    DOI: 10.1038/srep31796
    PMID: 27553888
  • Source: PubMed Central
    ProQuest Central
    DOAJ Directory of Open Access Journals

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