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Strategies in catalysts and electrolyzer design for electrochemical CO2 reduction toward C2+ products

Science advances, 2020-02, Vol.6 (8), p.eaay3111-eaay3111 [Peer Reviewed Journal]

Copyright © 2020 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC). 2020 The Authors ;EISSN: 2375-2548 ;DOI: 10.1126/sciadv.aay3111 ;PMID: 32128404

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  • Title:
    Strategies in catalysts and electrolyzer design for electrochemical CO2 reduction toward C2+ products
  • Author: Fan, Lei ; Xia, Chuan ; Yang, Fangqi ; Wang, Jun ; Wang, Haotian ; Lu, Yingying
  • Subjects: Electrochemistry ; Materials Science ; Review ; Reviews ; SciAdv reviews
  • Is Part Of: Science advances, 2020-02, Vol.6 (8), p.eaay3111-eaay3111
  • Description: Recent progress about electrochemical CO 2 reduction toward C 2+ products is reviewed. In light of environmental concerns and energy transition, electrochemical CO 2 reduction (ECR) to value-added multicarbon (C 2 + ) fuels and chemicals, using renewable electricity, presents an elegant long-term solution to close the carbon cycle with added economic benefits as well. However, electrocatalytic C─C coupling in aqueous electrolytes is still an open challenge due to low selectivity, activity, and stability. Design of catalysts and reactors holds the key to addressing those challenges. We summarize recent progress in how to achieve efficient C─C coupling via ECR, with emphasis on strategies in electrocatalysts and electrocatalytic electrode/reactor design, and their corresponding mechanisms. In addition, current bottlenecks and future opportunities for C 2 + product generation is discussed. We aim to provide a detailed review of the state-of-the-art C─C coupling strategies to the community for further development and inspiration in both fundamental understanding and technological applications.
  • Publisher: American Association for the Advancement of Science
  • Language: English
  • Identifier: EISSN: 2375-2548
    DOI: 10.1126/sciadv.aay3111
    PMID: 32128404
  • Source: PubMed Central
    DOAJ Directory of Open Access Journals
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